cv
Basics
| Name | Kirk A. Larsen |
| Label | Associate Scientist, Laser Sciences Department, Linac Coherent Light Source |
| larsenk@stanford.edu | |
| Url | https://profiles.stanford.edu/kirk-larsen |
| Summary | I am an associate scientist in the Laser Sciences Department at the Linac Coherent Light Source. I am generally interested in understanding how photon driven electronic motion and coherence in gas- and condensed-phase systems initiates chemical dynamics, charge transfer and energy transport. These processes can occur on few- to sub-femtosecond timescales (i.e. attoseconds). My research harnesses recent breakthroughs in ultrafast coherent light source development to gain insights into these processes. These advancements in light source technologies include both table-top lasers (nonlinear optics in hollow capillary fibers) and large-scale accelerators (advanced FEL modes and accelerator methods). |
Work
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2022.11 - Present Associate Scientist
Laser Sciences Department, Linac Coherent Light Source
Developing tunable few-cycle UV light sources using soliton dynamics and resonant dispersive wave emission in hollow capillary fibers. Primary contact for laser delivery and support at the coherent x-ray imaging (CXI) instrument at LCLS. Developing advanced photoinjector methods at LCLS for temporal x-ray pulse shaping and attosecond x-ray pulse generation at high repetition rates.
- Coherent X-ray Imaging Instrument, Linac Coherent Light Source - Laser Scientist POC and SLSO
- Ultrafast UV-Vis Sources Group, Laser Sciences Department - Tunable Few-Cycle Source Development
Education
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2021.01 - 2022.10 Stanford, CA
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2015.08 - 2020.12 Berkeley, CA
PhD
University of California, Berkeley
Applied Science and Technology
- Advisor: Professor Roger W. Falcone
- Thesis: Two-photon ionization and dissociation dynamics in atoms and molecules studied using vacuum ultraviolet laser harmonics and coincidence momentum imaging
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2009.09 - 2014.06 Eugene, OR
Volunteer
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2020.03 - Present -
2016.08 - 2019.12 -
2015.08 - 2019.12 Graduate Student Panel Member
Lawrence Berkeley National Laboratory, Workforce Development & Education
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2015.08 - 2015.12
Interests
| Science | |
| Atomic, molecular and optical physics | |
| Nonlinear optics | |
| Attosecond science | |
| Chemical physics | |
| Many-electron dynamics | |
| Non-adiabatic dynamics | |
| Electronic coherence | |
| Photoionization | |
| Photodissociation |
| Sources | |
| High harmonic generation | |
| Synchrotron radiation | |
| Free-electron lasers | |
| Spectral broadening and post-compression | |
| Bulk crystal harmonics | |
| Optical parametric amplification | |
| Optical solitons | |
| Resonant dispersive wave emission |
| Methods | |
| Coincidence momentum imaging | |
| Velocity map imaging | |
| Attosecond angular streaking | |
| Transient absorption spectroscopy | |
| Photoelectron spectroscopy | |
| Ultrafast soft x-ray spectroscopy | |
| Ultrafast hard x-ray scattering | |
| Ultrafast electron diffraction |
Projects
- 2022.11 - Present
Soliton dynamics and resonant dispersive wave emission in hollow capillary fibers
Generation and characterization of optical solitons and tunable few-cycle resonant dispersive waves in cascaded hollow capillary fibers driven by Yb laser systems.
- 2022.11 - Present
Coherent x-ray imaging at LCLS: laser developments
Expanding scientific scope at the coherent x-ray imaging instrument at LCLS through advanced laser techniques (e.g. spectral broadening and post-compression).
- 2021.01 - Present
Attosecond x-ray pump-probe spectroscopy at LCLS
Developing attosecond pulse generation methods at LCLS and performing attosecond x-ray pump + attosecond x-ray probe spectroscopy in gas- and condensed-phase systems.
- Science | DOI: 10.1126/science.adn6059
- Nature Photonics | DOI: 10.1038/s41566-024-01419-w
- Science Advances | DOI: 10.1126/sciadv.adp0841
- Physical Review X | DOI: 10.1103/PhysRevX.15.011008
- Nature Photonics | DOI: 10.1038/s41566-024-01427-w
- Physical Review Letters | DOI: 10.1103/PhysRevLett.134.115001
- Review of Scientific Instruments | DOI: 10.1063/5.0223334
- 2022.11 - Present
Megaelectronvolt Ultrafast Electron Diffraction (MeV-UED)
Tracking femtosecond electronic and structural dynamics in gas-phase atomic and molecular systems using ultrafast electron diffraction as a probe.
- 2022.11 - Present
Advanced photoinjector techniques: attosecond capabilities at high repetition rates
Developing advanced photoinjector methods at LCLS-II for temporal x-ray pulse shaping and attosecond x-ray pulse generation at high repetition rates.
- 2022.03 - 2023.09
Fresnel zone plate based soft x-ray photon spectrometer
Compact single-shot soft X-ray photon spectrometer for free-electron laser diagnostics.
- 2021.01 - Present
Attosecond light source and accelerator development at FACET-II
Developing attosecond XUV light sources and advanced accelerator methods at the Facility for Advanced Accelerator Experimental Tests (FACET-II).
- 2020.08 - 2021.09
SILIA: software implementation of a lock in amplifier
A software implementation of a lock in amplifier with an arbitrary number of channels and frequencies.
- 2015.08 - 2020.12
400 nm driven HHG: 3-D coincidence momentum imaging
Two-photon ionization and dissociation dynamics in isolated atoms and molecules studied using vacuum ultraviolet pulses produced via 400 nm driven high harmonic generation and coincidence momentum imaging.
- Physical Review A | DOI: 10.1103/PhysRevA.101.061402
- The Journal of Chemical Physics | DOI: 10.1063/5.0013485
- Physical Review A | DOI: 10.1103/PhysRevA.102.063118
- The Journal of Chemical Physics | DOI: 10.1063/5.0128846
- Physical Review Research | DOI: 10.1103/PhysRevResearch.3.033191 (800 nm driven HHG)
- 2015.08 - 2020.12
Advanced light source: 3-D coincidence momentum imaging
Single-photon single- and double-ionization and dissociation dynamics in isolated atoms and molecules studied using synchrotron radiation produced at the Advanced Light Source and coincidence momentum imaging.
- Physical Chemistry Chemical Physics | DOI: 10.1039/C8CP03637C
- Physical Review A | DOI: 10.1103/PhysRevA.99.043414
- Physical Review Research | DOI: 10.1103/PhysRevResearch.1.033140
- Physical Review Research | DOI: 10.1103/PhysRevResearch.2.043056
- Journal of Physics B: Atomic, Molecular and Optical Physics | DOI: 10.1088/1361-6455/abc3aa
- Nature Communications | DOI: 10.1038/s41467-022-32836-6
- Physical Chemistry Chemical Physics | DOI: 10.1039/D3CP02438E
- The Journal of Chemical Physics | DOI: 10.1063/5.0159300
- The Journal of Chemical Physics | DOI: 10.1063/5.0219029
- 2015.08 - 2019.03
800 nm driven HHG: velocity map imaging
The electronic and nuclear dynamics in methanol, following 156 nm photoexcitation, are investigated by combining a detailed analysis of time-resolved photoelectron spectroscopy experiments with electronic structure calculations.